Gutenberg Open Science: Nonequilibrium phase transition in an atomistic glassformer : the connection to thermodynamics

Please use this identifier to cite or link to this item: http://doi.org/10.25358/openscience-7174

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DC Field	Value	Language
dc.contributor.author	Turci, Francesco	-
dc.contributor.author	Royall, Patrick C.	-
dc.contributor.author	Speck, Thomas	-
dc.date.accessioned	2022-06-20T08:28:35Z	-
dc.date.available	2022-06-20T08:28:35Z	-
dc.date.issued	2017
dc.identifier.uri	https://openscience.ub.uni-mainz.de/handle/20.500.12030/7188	-
dc.description.abstract	Tackling the low-temperature fate of supercooled liquids is challenging due to the immense timescales involved, which prevent equilibration and lead to the operational glass transition. Relating glassy behaviour to an underlying, thermodynamic phase transition is a long-standing open question in condensed matter physics. Like experiments, computer simulations are limited by the small time window over which a liquid can be equilibrated. Here we address the challenge of low temperature equilibration using trajectory sampling in a system undergoing a emph{nonequilibrium} phase transition. This transition occurs in trajectory space between the normal supercooled liquid and a glassy state rich in low-energy geometric motifs. Our results indicate that this transition might become accessible in emph{equilibrium} configurational space at a temperature close to the so-called Kauzmann temperature, and provide a possible route to unify dynamical and thermodynamical theories of the glass transition.	en_GB
dc.description.sponsorship	DFG, Open Access-Publizieren Universität Mainz / Universitätsmedizin	de
dc.language.iso	eng	de
dc.rights	CC BY	*
dc.rights.uri	https://creativecommons.org/licenses/by/4.0/	*
dc.subject.ddc	530 Physik	de_DE
dc.subject.ddc	530 Physics	en_GB
dc.title	Nonequilibrium phase transition in an atomistic glassformer : the connection to thermodynamics	en_GB
dc.type	Zeitschriftenaufsatz	de
dc.identifier.doi	http://doi.org/10.25358/openscience-7174	-
jgu.type.dinitype	article	en_GB
jgu.type.version	Published version	de
jgu.type.resource	Text	de
jgu.organisation.department	FB 08 Physik, Mathematik u. Informatik	de
jgu.organisation.number	7940	-
jgu.organisation.name	Johannes Gutenberg-Universität Mainz	-
jgu.rights.accessrights	openAccess	-
jgu.journal.title	Physical review : X	de
jgu.journal.volume	7	de
jgu.journal.issue	3	de
jgu.pages.start	031028-1	de
jgu.pages.end	031028-14	de
jgu.publisher.year	2017	-
jgu.publisher.name	APS	de
jgu.publisher.place	College Park, Md.	de
jgu.publisher.uri	http://dx.doi.org/10.1103/PhysRevX.7.031028	de
jgu.publisher.issn	2160-3308	de
jgu.organisation.place	Mainz	-
jgu.subject.ddccode	530	de
opus.date.modified	2017-08-22T09:54:11Z
opus.subject.dfgcode	00-000
opus.organisation.string	FB 08: Physik, Mathematik und Informatik: Institut für Physik	de_DE
opus.identifier.opusid	57073
opus.institute.number	0801
opus.metadataonly	false
opus.type.contenttype	Keine	de_DE
opus.type.contenttype	None	en_EN
opus.affiliated	Speck, Thomas
jgu.publisher.doi	10.1103/PhysRevX.7.031028	de
jgu.organisation.ror	https://ror.org/023b0x485
Appears in collections:	DFG-OA-Publizieren (2012 - 2017)

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