Please use this identifier to cite or link to this item: http://doi.org/10.25358/openscience-5959
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dc.contributor.authorKneip, Nina-
dc.contributor.authorDüllmann, Christoph E.-
dc.contributor.authorGadelshin, Vadim-
dc.contributor.authorHeinke, Reinhard-
dc.contributor.authorMokry, Christoph-
dc.contributor.authorRaeder, Sebastian-
dc.contributor.authorRunke, Jörg-
dc.contributor.authorStuder, Dominik-
dc.contributor.authorTrautmann, Norbert-
dc.contributor.authorWeber, Felix-
dc.contributor.authorWendt, Klaus-
dc.date.accessioned2021-05-27T10:44:41Z-
dc.date.available2021-05-27T10:44:41Z-
dc.date.issued2020-
dc.identifier.urihttps://openscience.ub.uni-mainz.de/handle/20.500.12030/5968-
dc.description.abstractResonance ionization mass spectroscopy has proven to be a very efficient and selective method for the spatially resolved ultratrace determination of actinide contaminations, and the analysis of specific element and isotopic distributions on surfaces and environment particles. We report on the identification of highly element-selective optical excitation schemes identified for this purpose, with a particular focus on the precise determination of the isobaric ratios of 235U to 239Pu as well as 243Am to 241Pu. The chosen two-step ionization schemes were characterized with respect to their element selectivity on synthetic multi-element actinide mixtures, with an element ratio Pu : Am : U of 1 : 10 : 104, a composition which is typical, e.g., for spent nuclear reactor fuels.en_GB
dc.language.isoengde
dc.rightsCC BY*
dc.rights.urihttps://creativecommons.org/licenses/by/4.0/*
dc.subject.ddc530 Physikde_DE
dc.subject.ddc530 Physicsen_GB
dc.subject.ddc540 Chemiede_DE
dc.subject.ddc540 Chemistry and allied sciencesen_GB
dc.titleHighly selective two-step laser ionization schemes for the analysis of actinide mixturesen_GB
dc.typeZeitschriftenaufsatzde
dc.identifier.doihttp://doi.org/10.25358/openscience-5959-
jgu.type.dinitypearticleen_GB
jgu.type.versionPublished versionde
jgu.type.resourceTextde
jgu.organisation.departmentFB 08 Physik, Mathematik u. Informatikde
jgu.organisation.departmentFB 09 Chemie, Pharmazie u. Geowissensch.de
jgu.organisation.number7940-
jgu.organisation.number7950-
jgu.organisation.nameJohannes Gutenberg-Universität Mainz-
jgu.rights.accessrightsopenAccess-
jgu.journal.titleHyperfine interactionsde
jgu.journal.volume241de
jgu.pages.alternative45de
jgu.publisher.year2020-
jgu.publisher.nameSpringer Verlagde
jgu.publisher.urihttps://doi.org/10.1007/s10751-020-01712-4de
jgu.publisher.issn1572-9540de
jgu.organisation.placeMainz-
jgu.subject.ddccode530de
jgu.subject.ddccode540de
jgu.publisher.doi10.1007/s10751-020-01712-4
jgu.organisation.rorhttps://ror.org/023b0x485
Appears in collections:JGU-Publikationen

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