Gutenberg Open Science: Polyoxometalate-soft matter composite materials : design strategies, applications, and future directions

Please use this identifier to cite or link to this item: http://doi.org/10.25358/openscience-8782

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DC Field	Value	Language
dc.contributor.author	Kruse, Jan-Hendrik	-
dc.contributor.author	Langer, Marcel	-
dc.contributor.author	Romanenko, Iuliia	-
dc.contributor.author	Trentin, Ivan	-
dc.contributor.author	Hernández-Castillo, David	-
dc.contributor.author	González, Leticia	-
dc.contributor.author	Schacher, Felix H.	-
dc.contributor.author	Streb, Carsten	-
dc.date.accessioned	2023-02-09T09:43:12Z	-
dc.date.available	2023-02-09T09:43:12Z	-
dc.date.issued	2022	-
dc.identifier.uri	https://openscience.ub.uni-mainz.de/handle/20.500.12030/8798	-
dc.description.abstract	Molecular metal oxides or polyoxometalates (POMs) offer unrivaled properties in areas ranging from catalysis and energy conversion through to molecular electronics, biomimetics, and theranostics. While POMs are ubiquitous metal oxide model systems studied in most areas of chemistry and materials science, their technological deployment is often hampered by their molecular nature, as this leads to increased degradation, leaching, and loss of reactivity, particularly when harsh applications, such as water electrolysis, thermal catalysis or highly basic/acidic reaction solutions are targeted. Therefore, immobilization of POMs on heterogeneous substrates has recently become a central theme in POM research. While early studies focused mainly on metal oxide and semiconductor supports, more recently, POM integration in soft matter matrices including polymers, conductive polymers, hydrogels, and stimuli-responsive matrices leads to breakthroughs in multifunctional composite design. This Review summarizes pioneering experimental and theoretical progress in this emerging field over the last decade, highlighting current challenges that need to be overcome to allow a more widespread technological deployment and providing the authors’ view of some of the most promising future directions of the research field. In addition, the current understanding of correlations between structure (on the molecular, nano- and microscale) and reactivity in POM polymer composites is summarized, so that rational materials design can be further developed.	en_GB
dc.description.sponsorship	Gefördert durch die Deutsche Forschungsgemeinschaft (DFG) - Projektnummer 491381577	de
dc.language.iso	eng	de
dc.rights	CC BY	*
dc.rights.uri	https://creativecommons.org/licenses/by/4.0/	*
dc.subject.ddc	540 Chemie	de_DE
dc.subject.ddc	540 Chemistry and allied sciences	en_GB
dc.title	Polyoxometalate-soft matter composite materials : design strategies, applications, and future directions	en_GB
dc.type	Zeitschriftenaufsatz	de
dc.identifier.doi	http://doi.org/10.25358/openscience-8782	-
jgu.type.dinitype	article	en_GB
jgu.type.version	Published version	de
jgu.type.resource	Text	de
jgu.organisation.department	FB 09 Chemie, Pharmazie u. Geowissensch.	de
jgu.organisation.number	7950	-
jgu.organisation.name	Johannes Gutenberg-Universität Mainz	-
jgu.rights.accessrights	openAccess	-
jgu.journal.title	Advanced functional materials	de
jgu.journal.volume	32	de
jgu.journal.issue	51	de
jgu.pages.alternative	2208428	de
jgu.publisher.year	2022	-
jgu.publisher.name	Wiley-Blackwell	de
jgu.publisher.place	Weinheim	de
jgu.publisher.issn	1616-3028	de
jgu.organisation.place	Mainz	-
jgu.subject.ddccode	540	de
jgu.publisher.doi	10.1002/adfm.202208428	de
jgu.organisation.ror	https://ror.org/023b0x485	-
jgu.subject.dfg	Naturwissenschaften	de
Appears in collections:	DFG-491381577-H

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